Ba+2 ion trapping using organic submonolayer for ultra-low background neutrinoless double beta detector

使用有机亚单层捕获 Ba+2 离子以实现超低背景无中微子双 beta 探测器

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作者:P Herrero-Gómez, J P Calupitan, M Ilyn, A Berdonces-Layunta, T Wang, D G de Oteyza, M Corso, R González-Moreno, I Rivilla, B Aparicio, A I Aranburu, Z Freixa, F Monrabal, F P Cossío, J J Gómez-Cadenas, C Rogero; NEXT collaboration

Abstract

If neutrinos are their own antiparticles the otherwise-forbidden nuclear reaction known as neutrinoless double beta decay can occur. The very long lifetime expected for these exceptional events makes its detection a daunting task. In order to conduct an almost background-free experiment, the NEXT collaboration is investigating novel synthetic molecular sensors that may capture the Ba dication produced in the decay of certain Xe isotopes in a high-pressure gas experiment. The use of such molecular detectors immobilized on surfaces must be explored in the ultra-dry environment of a xenon gas chamber. Here, using a combination of highly sensitive surface science techniques in ultra-high vacuum, we demonstrate the possibility of employing the so-called Fluorescent Bicolor Indicator as the molecular component of the sensor. We unravel the ion capture process for these molecular indicators immobilized on a surface and explain the origin of the emission fluorescence shift associated to the ion trapping.

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