The enrichment ratio of atomic contacts in the crystal structure of isomeric, triply protonated, 4'-functionalized terpyridine cations with [ZnCl(4)](2-) as counter-ion

以[ZnCl(4)](2-)为抗衡离子的异构体、三质子化、4'-官能化的三联吡啶阳离子晶体结构中原子接触的富集比

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Abstract

We report herein the synthesis, crystallographic analysis and a study of the non-covalent inter-actions observed in the new 4'-substituted terpyridine-based derivative bis-[4'-(isoquinolin-2-ium-4-yl)-4,2':6',4''-terpyridine-1,1''-diium] tris-[tetra-chlorido-zincate(II)], (C(24)H(19)N(4))(2)[ZnCl(4)](3) or (44TPH(3))(2)[ZnCl(4)](3), where (44TPH(3))(3+) is the triply protonated cation 4'-(isoquinolinium-4-yl)-4,2':6',4'' terpyridinium. The compound is similar in its formulation to the recently reported 2,2':6',2'' terpyridinium analogue {bis-[4'-(isoquinolin-2-ium-4-yl)-2,2':6',2''-terpyridine-1,1''-diium] tris-[tetra-chlorido-zincate(II)] monohydrate; Granifo et al. (2017 ▸). Acta Cryst. C73, 1121-1130}, although rather different and much simpler in its structural features, mainly in the number and type of non-covalent inter-actions present, as well as in the supra-molecular structure they define.

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