Fabrication of a novel electrochemical sensor for determination of hydrogen peroxide in different fruit juice samples

制备一种新型电化学传感器用于测定不同果汁样品中的过氧化氢含量

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Abstract

A new hydrogen peroxide (H(2)O(2)) sensor is fabricated based on a multiwalled carbon nanotube-modified glassy carbon electrode (MWCNT-GCE) and reactive blue 19 (RB). The charge transfer coefficient, α, and the charge transfer rate constant, k(s), of RB adsorbed on MWCNT-GCE were calculated and found to be 0.44 ± 0.01 Hz and 1.9 ± 0.05 Hz, respectively. The catalysis of the electroreduction of H(2)O(2) by RB-MWCNT-GCE is described. The RB-MWCNT-GCE shows a dramatic increase in the peak current and a decrease in the overvoltage of H(2)O(2) electroreduction in comparison with that seen at an RB modified GCE, MWCNT modified GCE, and activated GCE. The kinetic parameters such as α and the heterogeneous rate constant, k', for the reduction of H(2)O(2) at RB-MWCNT-GCE surface were determined using cyclic voltammetry. The detection limit of 0.27μM and three linear calibration ranges were obtained for H(2)O(2) determination at the RB-MWCNT-GCE surface using an amperometry method. In addition, using the newly developed sensor, H(2)O(2) was determined in real samples with satisfactory results.

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