Vinylidenation of Organoboronic Esters Enabled by a Pd-Catalyzed Metallate Shift

钯催化金属酸盐迁移实现有机硼酸酯的乙烯基化反应

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Abstract

Organoboron "ate" complexes undergo a net vinyl insertion reaction to give 1,1-disubstituted alkenyl boronic esters when treated with stoichiometric allyl acetate and a palladium catalyst. Reactions that employ vinyllithium afforded good to excellent yields after one hour, while reactions that employ vinylmagnesium chloride furnished modest to good yields after 18 hours.

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