Sequential C(sp3)-H arylation and olefination: total synthesis of the proposed structure of pipercyclobutanamide A

顺序 C(sp3)-H 芳基化和烯烃化:哌啶环丁酰胺 A 的拟议结构的合成

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Abstract

A strategy for assembling tetrasubstituted cyclobutanes is reported in the context of a short, protecting-group-free synthesis of the proposed structure of pipercyclobutanamide A. The route features sequential C–H functionalizations on an unactivated cyclobutane wherein C–C bonds to aryl and styrenyl groups are made one-by-one in a stereocontrolled fashion.

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