Abstract
This study explores the development of biodegradable starch-based films treated with dielectric barrier discharge (DBD) plasma and incorporated with acerola residue and grape pomace extracts. The primary aim was to enhance the films' physicochemical properties and introduce pH-sensing capabilities. Plasma treatment at 200 Hz for 20 min modified the films' amylose content (by 13.2%), solubility (by 13.3%), contact angle (by 12.7%), moisture content (by 14.2%), and surface morphology. The addition of the extracts changed the short-range ordered structure parameters of the films (by 111.4%), solubility (by 11.1%), moisture content (by 18.4%), and water vapor permeability (by 6.1%). The films with acerola residue and grape pomace extracts exhibited good colorimetric responses for pH indication. The films with acerola residue extract tended to intensify the yellowish color, while those with grape pomace extract showed more significant color changes varying from purple to green. Integrating natural pigments like anthocyanins from grape pomace and carotenoids from acerola improved the films' functional properties and provided a visual indication of food freshness through pH changes.