Antiproliferative activity of Xylopia aethiopica extracts and molecular docking studies of their main phytochemicals

非洲爪哇木提取物的抗增殖活性及其主要植物化学成分的分子对接研究

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Abstract

Xylopia aethiopica (African pepper) is an intriguing medicinal plant which grows abundantly in West Africa and demonstrates a variety of pharmacological properties. This study assesses the cytotoxic activity of hexane, ethyl acetate and methanol extracts of the fruits and root of the plant against HCC-70, MCF-7, and MCF12A cell lines. The ethyl acetate fraction of the root had the strongest cytotoxic activity against HCC-70, a highly aggressive Triple-Negative Breast Cancer (TNBC) cell line, with an IC(50) of 19.96 µg/mL. The hexane extract of the fruit had an IC(50) value of 30.39 µg/mL against MCF-7. The cytotoxic effects observed could be attributed to a wide spectrum of phytochemicals in the extracts. Using the fingerprint pattern from the (13)C-NMR of the extracts, seven compounds belonging to two classes (i.e., kaurene and trachylobane-type diterpenoids and aporphine-type alkaloids) were annotated from the extracts. Furthermore, these compounds were assessed in silico on several important tumour cell-associated proteins. Two compounds showcased excellent binding interactions across all the proteins investigated and displayed a favourable ADMET profile. N-methylnordomesticine and N-methyllaurotetanine are excellent leads for further medicinal chemistry development. SUPPLEMENTARY INFORMATION: The online version contains supplementary material available at 10.1007/s40203-026-00633-4.

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