Abstract
Investigating valley-related physics in rare intrinsic ferromagnetic materials with high-temperature stability and viable synthesis methods is of vital importance for advancing fundamental physics and information technology. Through first-principles calculations, we forecast that monolayer TiAlTe(3) has superb structural stability, a ferromagnetic coupling mechanism deriving from direct-exchange and superexchange interactions, and a high magnetic transition temperature. We observed spontaneous valley polarization of 103 meV in the bottom conduction band when monolayer TiAlTe(3) is magnetized toward an out-of-plane orientation. Additionally, because of its powerful valley-contrasting Berry curvature, the anomalous valley Hall effect emerges under an in-plane electric field. The cooperation of ferromagnetic coupling, a high magnetic transition temperature, and spontaneous valley polarization makes monolayer TiAlTe(3) a promising room-temperature ferrovalley material for use in nanoscale spintronics and valleytronics.