Ajwa Date Seed-Derived Hydrogel Electrolyte with Enhanced Electrochemical Performance and Mechanical Strength for Flexible Supercapacitors

用于柔性超级电容器的具有增强电化学性能和机械强度的阿吉瓦枣籽衍生水凝胶电解质

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Abstract

Background: The growing demand for sustainable, high-performance energy storage systems has intensified interest in biomass-derived materials for supercapacitor applications. This study presents a green and scalable approach to fabricating novel electrodes and solid-state electrolytes using Phoenix dactylifera (Ajwa date) seed biomass and palm waste-derived activated carbon. Methods: KOH-activated carbon from date pits was employed to enhance surface area and redox activity. A double-network hydrogel electrolyte (DSHC) was synthesized by incorporating 0.5 g of date seed powder with sodium alginate and wheat starch (0.2 g each), followed by chemical crosslinking in 2 M H(2)SO(4). Structural and physicochemical properties were analyzed using SEM, XRD, and FTIR, while electrochemical performance was evaluated through cyclic voltammetry and galvanostatic charge-discharge measurements. Results: SEM revealed a densely ordered porous network with regular cylindrical channels favorable for ion transport. XRD and FTIR confirmed amorphous carbon formation and effective molecular crosslinking. The hydrogel electrolyte exhibited a wide potential window of ~2 V and strong pseudocapacitive behavior, delivering a maximum specific capacitance of 179 F g(-1) at 5 mV s(-1) and a discharge capacitance of 159 F g(-1) at 0.2 A g(-1), with excellent stability over 5500 cycles. Conclusions: Agricultural waste-derived materials demonstrate strong potential as low-cost, eco-friendly, and mechanically robust components for flexible supercapacitors, suitable for sustainable energy storage and rapid-charging applications.

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