Linamarin and its analogues as targeted therapeutic agents in cervical cancer: insights from atomistic molecular docking, dynamics and MMPBSA calculations

利那马林及其类似物作为宫颈癌靶向治疗药物:来自原子分子对接、动力学和MMPBSA计算的启示

阅读:2

Abstract

The HPV16 E6 oncoprotein is a critical target for therapeutic intervention in cervical cancerIn this study, we investigated the interactions of linamarin and its analogues ZINC146037704, ZINC141150528 and ZINC146038957 with HPV16 E6 protein using molecular docking, dynamics, MMPBSA and ADMET predictions. Docking and MD confirmed ZINC146037704 analogue as the most favourable binding candidate with the lowest binding free energy (-74.93 ± 13.05 kJ/mol), stable RMSD (≈0.35 nm) and Rg (2.1988 nm) values, and the highest number of hydrogen bonds (14), indicating strong and persistent ligand-protein interactions. Per-residue decomposition highlighted key contributions from sub-interface I, II, LxxL motif consistent with critical residues in E6-p53 interface stabilization. Ligand interactions were primarily mediated by hydrogen bonds, π-stacking, and van der Waals forces, with glycosylated moieties enhancing polar contacts and binding stability compared to the control drug, topotecan. ADMET evaluation indicated generally favourable pharmacokinetic and safety profiles, with ZINC146037704 and ZINC3984017 showing balanced properties for further development. Overall, these results identify ZINC146037704 as a promising lead molecule for targeting HPV16 E6 and provide a foundation for future experimental validation of linamarin-derived inhibitors in cervical cancer therapy. SUPPLEMENTARY INFORMATION: The online version contains supplementary material available at 10.1007/s40203-026-00619-2.

特别声明

1、本页面内容包含部分的内容是基于公开信息的合理引用;引用内容仅为补充信息,不代表本站立场。

2、若认为本页面引用内容涉及侵权,请及时与本站联系,我们将第一时间处理。

3、其他媒体/个人如需使用本页面原创内容,需注明“来源:[生知库]”并获得授权;使用引用内容的,需自行联系原作者获得许可。

4、投稿及合作请联系:info@biocloudy.com。