Two-Dimensional Spectroscopy of Open Quantum Systems: Nonequilibrium Green's Function Formulation

开放量子系统的二维光谱学:非平衡格林函数形式

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Abstract

Two-dimensional spectroscopy is examined for open quantum systems featuring multiple simultaneously measurable fluxes. Specifically, we explore a junction where optical measurements of photon flux are paired with concurrent transport measurements of electron currents. The theory of two-dimensional spectroscopy for both fluxes is developed using a nonself-consistent nonequilibrium Green's function formulation. Theoretical derivations are demonstrated through numerical simulations within a generic junction model.

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