Abstract
We demonstrate by use of continuous wave- and pulse-electron paramagnetic resonance spectroscopy on oriented single crystals of magnetically dilute Yb(III) ions in Yb(0.01)Lu(0.99)(trensal) that molecular entangled two-qubit systems can be constructed by exploiting dipolar interactions between neighboring Yb(III) centers. Furthermore, we show that the phase memory time and Rabi frequencies of these dipolar-interaction-coupled entangled two-qubit systems are comparable to the ones of the corresponding single qubits.