Plasmon-Enhanced Visible and Near-Infrared Photodetection with Gold Nanorods UCNPs/MoS(2) Hybrid Device

利用金纳米棒上转换纳米粒子/二硫化钼混合器件实现等离子体增强的可见光和近红外光电探测

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Abstract

The near-infrared photodetection of monolayer MoS(2) can be achieved using upconverted nanoparticles (UCNPs). Herein, we demonstrated that gold nanorods (Au NRs) further enhanced the near-infrared photoresponsivity of a hybrid device via the surface plasmon enhancement of the localized field. We synthesized a three-layer device comprising Au NRs, UCNPs (NaYF(4):Yb(3+), Er(3+)), and monolayer MoS(2), and examined its photoelectric characteristics using laser irradiation with varying power densities at 980 nm, the excitation wavelength of UCNPs. Compared with a device without Au NRs, the photoelectric response of the three-layer device was greatly improved at 5 V bias, and photoresponsivity was increased at visible wavelengths (450, 532, and 635 nm). This study contributes to the knowledge of two-dimensional materials for the development of hybrid photoelectronic devices.

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