Crystal structure and Hirshfeld surface analysis of mono/bis-(aqua-κO)[N-(2-oxido-benzyl-idene)valinato-κ(3) O,N,O']copper(II): dimeric Schiff base copper(II) complexes having different numbers of coordinated water mol-ecules

单/双-(水-κO)[N-(2-氧化苄基亚甲基)缬氨酸-κ(3)O,N,O']铜(II)配合物的晶体结构和Hirshfeld表面分析:具有不同数量配位水分子的二聚席夫碱铜(II)配合物

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Abstract

The mol-ecular structure of the title compound, [Cu(C(12)H(13)N(2)O(3))(H(2)O)(2)]·[Cu(C(12)H(13)N(2)O(3))(H(2)O)], consists of two different mol-ecules in the asymmetric unit. Both of the structures consist of a tridentate ligand synthesized from l-valine and salicyl-aldehyde, and one water mol-ecule or two water mol-ecules coordinating to Cu(II). They have a square-planar (mol-ecule 1) or a square-pyramidal (mol-ecule 2) coordination geometry. In the crystal, the mol-ecules form intra- and inter-molecular O-H⋯O hydrogen bonds involving the coordinated water mol-ecules and other sites. A Hirshfeld surface analysis indicated that the most important contributions to the packing are from H⋯H [52.9% (mol-ecule 1) and 51.1% (mol-ecule 2)] and H⋯O/ O⋯H [21.2% (mol-ecule 1) and 25.8% (mol-ecule 2)] contacts. In addition, an electrostatic potential map was also obtained from DFT calculations to support the discussion of the inter-molecular inter-actions.

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