Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields

磁场调控单层过渡金属二硫化物中的双激子

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Abstract

We present time-integrated four-wave mixing measurements on monolayer MoSe(2) in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fields the coherence at negative and positive time delays is dominated by intervalley biexcitons. We demonstrate that magnetic fields can serve as a control to enhance the biexciton formation and help search for more exotic states of matter, including the creation of multiple exciton complexes and excitonic condensates.

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