Synthesis of C14-C21 acid fragments of cytochalasin Z(8) via anti-selective aldol condensation and B-alkyl Suzuki-Miyaura cross-coupling

通过反选择性羟醛缩合和β-烷基Suzuki-Miyaura交叉偶联反应合成细胞松弛素Z(8)的C14-C21酸片段

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Abstract

An efficient synthesis of the C14-C21 acid fragment of cytochalasin Z(8) was accomplished in 10 steps with 14% overall yield. Boron-mediated anti-selective aldol condensation and Pd(OAc)(2)-Aphos-Y-catalysed B-alkyl Suzuki-Miyaura cross-coupling were employed to construct the requisite C17 and C18 stereogenic centres and alkene subunit.

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