Processing and Characterization of Spent Nickel-Metal Hydride Type AA Batteries to Recover Valuable Materials (Cobalt, Nickel and Rare Earth Elements)

废旧镍氢AA型电池的处理和表征,以回收有价值的材料(钴、镍和稀土元素)

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Abstract

The experimental research was focused on the investigation of valuable material from spent Ni-MH type AA batteries, namely the metal grid anodes and the black mass material (anode and cathode powder). The materials of interest were analyzed by X-ray fluorescence spectroscopy (XRF), ICP-OES (inductively coupled plasma optical emission spectrometry), optical microscopy, scanning electron microscopy (SEM), energy-dispersive X-ray analysis (EDX), electron backscatter diffraction (EBSD), and X-ray diffraction (XRD). The analyzed grids have a high Fe content, but some of them correspond to the Invar alloy with approx. 40% Ni. In the black mass material, round particles and large aggregations were observed by SEM analysis, showing a high degree of degradation. The XRD analysis reveals the presence of only three compounds or phases that crystallize in the hexagonal system: La(0.52)Ce(0.33)Pr(0.04)Nd(0.11)Co(0.6)Ni(4.4), Ni(OH)(2), and La(5)Ni(19). The obtained results provide useful and interesting information that can be used for further research in the recycling and economic assessment of metals from spent Ni-MH batteries.

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