Microscopic Theory of Energy Dissipation and Decoherence in Solid-State Quantum Devices: Need for Nonlocal Scattering Models

固态量子器件中能量耗散和退相干的微观理论:对非局域散射模型的需求

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Abstract

Energy dissipation and decoherence in state-of-the-art quantum nanomaterials and related nanodevices are routinely described and simulated via local scattering models, namely relaxation-time and Boltzmann-like schemes. The incorporation of such local scattering approaches within the Wigner-function formalism may lead to anomalous results, such as suppression of intersubband relaxation, incorrect thermalization dynamics, and violation of probability-density positivity. The primary goal of this article is to investigate a recently proposed quantum-mechanical (nonlocal) generalization (Phys. Rev. B 2017, 96, 115420) of semiclassical (local) scattering models, extending such treatment to carrier-carrier interaction, and focusing in particular on the nonlocal character of Pauli-blocking contributions. In order to concretely show the intrinsic limitations of local scattering models, a few simulated experiments of energy dissipation and decoherence in a prototypical quantum-well semiconductor nanostructure are also presented.

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