Growth of α-Ga(2)O(3) from Gallium Acetylacetonate under HCl Support by Mist Chemical Vapor Deposition

采用雾化化学气相沉积法,以乙酰丙酮镓为前驱体,在HCl载体上生长α-Ga₂O₃

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Abstract

α-Ga(2)O(3) films were grown on a c-plane sapphire substrate by HCl-supported mist chemical vapor deposition with multiple solution chambers, and the effect of HCl support on α-Ga(2)O(3) film quality was investigated. The growth rate monotonically increased with increasing Ga supply rate. However, as the Ga supply rate was higher than 0.1 mmol/min, the growth rate further increased with increasing HCl supply rate. The surface roughness was improved by HCl support when the Ga supply rate was smaller than 0.07 mmol/min. The crystallinity of the α-Ga(2)O(3) films exhibited an improvement with an increase in the film thickness, regardless of the solution preparation conditions, Ga supply rate, and HCl supply rate. These results indicate that there is a low correlation between the improvement of surface roughness and crystallinity in the α-Ga(2)O(3) films grown under the conditions described in this paper.

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