Microscopic probing of the superconducting and normal state properties of Ta(2)V(3.1)Si(0.9) by muon spin rotation

利用μ子自旋旋转对Ta(2)V(3.1)Si(0.9)的超导和正常态性质进行微观探测

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Abstract

The two-dimensional kagome lattice is an experimental playground for novel physical phenomena, from frustrated magnetism and topological matter to chiral charge order and unconventional superconductivity. A newly identified kagome superconductor, Ta(2)V(3.1)Si(0.9) has recently gained attention for possessing a record high critical temperature, T (C) = 7.5 K for kagome metals at ambient pressure. In this study we conducted a series of muon spin rotation measurements to delve deeper into understanding the superconducting and normal state properties of Ta(2)V(3.1)Si(0.9). We demonstrate that Ta(2)V(3.1)Si(0.9) is a bulk superconductor with either a s+s-wave or anisotropic s-wave gap symmetry, and has an unusual paramagnetic shift in response to external magnetic fields in the superconducting state. Additionally, we observe an exceptionally low superfluid density - a distinctive characteristic of unconventional superconductivity - which remarkably is comparable to the superfluid density found in hole-doped cuprates. In its normal state, Ta(2)V(3.1)Si(0.9) exhibits a significant increase in the zero-field muon spin depolarisation rate, starting at approximately 150 K, which has been observed in other kagome-lattice superconductors, and therefore hints at possible hidden magnetism. These findings characterise Ta(2)V(3.1)Si(0.9) as an unconventional superconductor and a noteworthy new member of the vanadium-based kagome material family.

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