Effect of Printing Temperature on the Microstructure and Tensile Properties of Polylactic Acid-Magnetic Iron Composites Manufactured by Material Extrusion

打印温度对挤出成型聚乳酸-磁性铁复合材料的微观结构和拉伸性能的影响

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Abstract

In this study, we examined how printing temperature affects the microstructure and mechanical properties of polylactic acid (PLA) composite reinforced with iron oxide i.e., magnetite manufactured using a material extrusion technique. The composite was printed at temperatures from 185 °C to 215 °C. Microstructure analysis via synchrotron radiation X-ray microtomography revealed changes in both iron oxide and porosity contents within the printed structures. Mechanical testing results demonstrated a limited effect of the printing temperature on tensile performance. Finite element computation is considered to predict the elasticity behavior of the printed composite by converting 3D images into 3D structural meshes. When implementing a two-phase model, the predictions show a leading role of the iron oxide content, and an overestimation of the stiffness of the composite. A three-phase model demonstrates a better matching of the experimental results suggesting a limited load transfer across the PLA-iron oxide interface with Young's moduli in the interphase zone as small as 10% of PLA Young's modulus. Magnetic actuation demonstrates that experiments on PLA-iron oxide plates reveal a pronounced thickness-dependent limitation, with the maximum deflection observed in thin strips of 0.4 mm.

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