Plasmon-exciton couplings in the MoS2/AuNP plasmonic hybrid structure

MoS2/AuNP 等离子体混合结构中的等离子体-激子耦合

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作者:Hyuntae Kim #, Jaeseung Im #, Kiin Nam, Gang Hee Han, Jin Young Park, Sungjae Yoo, MohammadNavid Haddadnezhad, Sungho Park, Woongkyu Park, Jae Sung Ahn, Doojae Park, Mun Seok Jeong, Soobong Choi

Abstract

The understanding and engineering of the plasmon-exciton coupling are necessary to control the innovative optoelectronic device platform. In this study, we investigated the intertwined mechanism of each plasmon-exciton couplings in monolayer molybdenum disulfide (MoS2) and plasmonic hybrid structure. The results of absorption, simulation, electrostatics, and emission spectra show that interaction between photoexcited carrier and exciton modes are successfully coupled by energy transfer and exciton recombination processes. Especially, neutral exciton, trion, and biexciton can be selectively enhanced by designing the plasmonic hybrid platform. All of these results imply that there is another degree of freedom to control the individual enhancement of each exciton mode in the development of nano optoelectronic devices.

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