High-Quality Perovskite CH₃NH₃PbI₃ Thin Films for Solar Cells Prepared by Single-Source Thermal Evaporation Combined with Solvent Treatment

单源热蒸发结合溶剂处理制备太阳能电池用高品质钙钛矿 CH₃NH₃PbI₃ 薄膜

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作者:Huanxin Peng, Zhenghua Su, Zhuanghao Zheng, Huabin Lan, Jingting Luo, Ping Fan, Guangxing Liang

Abstract

In this work, solvent annealing process for CH&sub3;NH&sub3;PbI&sub3; thin film prepared by single source evaporation was reported. Characterized by the scanning electron microscope (SEM), X-ray diffractometer (XRD), energy dispersive spectroscope (EDS), ultraviolet-visible (UV) spectrophotometer, and the photoluminescence (PL) spectrometer, our method ensured higher quality film with crystallinity, composition, well-defined grain structure, and reproducibility. The optimized solar cell device based on the structure of ITO/PEDOT:PSS/CH&sub3;NH&sub3;PbI&sub3;/PCBM/Ag achieved better performance in power conversion efficiency from 2.64% to 9.92%, providing an effective method to optimize the quality of perovskite film for solar cell application.

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