Fluorescent Zn(II) Chemosensor Mediated by a 1,8-Naphthyridine Derivative and It's Photophysical Properties

1,8-萘啶衍生物介导的荧光锌(II)化学传感器及其光物理性质

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Abstract

One of the greatest challenges in using fluorescent chemosensors for highly selective and sensitive transition-metal ions is finding an efficient and simple method for its synthesis. In this study, a highly efficient fluorescence chemosensor for Zn(II) was developed from N-Boc-L-proline modified 1,8-naphthyridine. The fluorescence intensity of the chemosensor was increased significantly only in the presence of Zn(II) ion which provided a perceived color change for rapid visual sensing, while other metal ions showed fluorescence quenching or little changes. It was worth noting that the chemosensor L distinguished Zn(II) from Cd(II) commonly having similar properties. The solvent effect and possible bonding mode for fluorescence enhancement have been also discussed. Results of this study indicated that the Boc-group in l-proline significantly improved the sensitivity and selectivity for Zn(II) detection performance, as confirmed by comparison experiments and time dependent-density functional theory (TD-DFT) calculations.

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