Abstract
Soliton molecules, or also known as optical bound states, are the most representative example of solitons' particle nature and have given birth to diverse light-matter analogies. Despite detailed research on regular bound states, the soliton molecule synthesis of dissimilar pulses has rarely been reported. Here, soliton molecules formed by dissimilar dissipative solitons are demonstrated in a single-mode mode-locked fiber laser, with an in-depth analysis of their evolution dynamics. This novel bound state features pulse trapping between two ultrafast vector pulses with distinct pulse properties including energy, duration, and chirp, leading to unique temporal and spectral profiles. This laser provides an optimal platform for studying complex interactions between different types of dissipative solitons. The findings here can provide new degrees of freedom for the generation of optical soliton molecules and can fuel applications in optical information processing, metrology, and spectroscopy.