Integrated Management of Bacterial Wilt and Root-Knot Nematode Diseases in Pepper: Discovery of Phenazine-1-Carboxamide from Pseudomonas aeruginosa W-126

辣椒细菌性枯萎病和根结线虫病的综合防治:从铜绿假单胞菌W-126中发现吩嗪-1-甲酰胺

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Abstract

Ralstonia solanacearum is an important pathogen causing bacterial wilt in pepper (Capsicum annuum L.). The concurrent infection of R. solanacearum and root-knot nematodes (Meloidogyne spp.) exacerbates the severity of bacterial wilt in pepper. Utilizing plant endophytic bacteria to control these mixed diseases is a viable strategy. Waltheria indica L. (Sterculiaceae) is a traditional medicine plant. A total of 209 endophytic bacteria were isolated from W. indica, and Pseudomonas aeruginosa W-126 showed an efficient antagonistic effect against R. solanacearum. Based on active compound tracking principles, a compound was isolated through silica gel column chromatography and preparative HPLC combined with TLC analysis. It was identified as phenazine-1-carboxamide (PCN) by spectral techniques (ESI-MS, (1)H-NMR, (13)C-NMR). PCN displayed excellent inhibitory activity against R. solanacearum, with an EC(50) of 64.16 μg/mL in vitro. In addition, it showed certain nematocide activity, with an LC(50) value of 118.63 μg/mL at 72 h. PCN also showed certain inhibitory activity against five other phytopathogenic bacteria. The structure-activity relationship indicated that the phenazine skeleton and acylamide groups were the key pharmacophores for the activity of phenazine-related compounds against R. solanacearum. PCN controlled the complex diseases of R. solanacearum and M. incognita in a pot experiment, with respective 51.41 and 39.80% inhibitory rates. The exploration of secondary metabolites of biocontrol bacteria can provide reference for the development of novel and efficient pesticides.

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