Simultaneous Determination and Dietary Risk Assessment of 26 Pesticide Residues in Wheat Grain and Bran Using QuEChERS-UHPLC-MS/MS

利用 QuEChERS-UHPLC-MS/MS 同时测定小麦籽粒和麸皮中 26 种农药残留并进行膳食风险评估

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Abstract

Evaluating the potential chronic health risks posed by pesticides to consumers is essential for ensuring food safety and protecting public health. An ultra-high-performance liquid chromatography-tandem mass spectrometry (UHPLC-MS/MS) method coupled with modified QuEChERS extraction was developed to simultaneously determine 26 pesticide residues in wheat grain and bran. Samples were extracted with acetonitrile with 2% (v/v) acetic acid and cleaned up using C(18) sorbent. Method validation demonstrated excellent linearity, accuracy, and precision. When applied to 48 wheat grain and 24 bran samples collected from major wheat-growing regions in China, 12 and 21 pesticides were detected at concentrations ranging from <0.005 to 1.785 mg kg(-1) and <0.01 to 2.188 mg kg(-1), respectively. Chronic hazard quotients (HQc) and acute hazard quotients (HQa) for all pesticides for grain and bran were far below the safety threshold of 100%. These results indicate that pesticide residues in wheat grain and bran present negligible chronic dietary risks to consumers across all age groups.

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