Efficient production of glycine from glucose via a two-stage biosynthetic strategy

通过两阶段生物合成策略高效地利用葡萄糖生产甘氨酸

阅读:1

Abstract

BACKGROUND: High-quality glycine is widely used in the cosmetics and pharmaceutical industries. Conventional chemical synthesis of glycine is disfavored because it relies on toxic reagents and complex downstream purification. RESULTS: Herein, we established an efficient two-step biosynthetic process for producing glycine from glucose. First, an l-threonine−overproducing strain was used to synthesis l-threonine via 50 L fed-batch fermentation, achieving a titer of 119.3 g/L. Then, a highly active l-threonine aldolase (PpLTA) was screened to convert l-threonine into glycine. To overcome thermodynamic and acetaldehyde inhibition constraints, an acetaldehyde elimination system was constructed via introducing ScADH1 and ScCR, which increased the molar conversion yield of glycine increased by 3.9-fold. Whole-cell catalysis gave a significantly higher conversion yield than crude enzyme preparations. A whole-cell co-expressing PpLTA, ScADH1, and ScCR was subsequently constructed. Finally, at 50 L scale, direct conversion of l-threonine fermentation broth afforded a glycine titer of 65.4 g/L within 24 h, with a molar conversion yield of 87.2%, In addition, 99.8% pure glycine was obtained with a yield of 76.6% via separation. CONCLUSIONS: An efficient two-step process for converting glucose to glycine was developed and successfully validated. Evaluation at the 50 L scale demonstrated record-high glycine production performance. This work provides a promising technological route for the industrial manufacture of high-quality glycine. GRAPHICAL ABSTRACT: [Image: see text] SUPPLEMENTARY INFORMATION: The online version contains supplementary material available at 10.1186/s12934-026-02966-3.

特别声明

1、本页面内容包含部分的内容是基于公开信息的合理引用;引用内容仅为补充信息,不代表本站立场。

2、若认为本页面引用内容涉及侵权,请及时与本站联系,我们将第一时间处理。

3、其他媒体/个人如需使用本页面原创内容,需注明“来源:[生知库]”并获得授权;使用引用内容的,需自行联系原作者获得许可。

4、投稿及合作请联系:info@biocloudy.com。