Hard-templating of chiral TiO(2) nanofibres with electron transition-based optical activity

基于电子跃迁光学活性的手性TiO₂纳米纤维的硬模板法

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Abstract

The fabrication of optically active inorganic nanomaterials with chiral superstructures attracts attention because of their potential applications in chemical sensing and non-linear optics. Here, we present a facile way to prepare TiO(2) nanofibres, in which the nanocrystals are helically arranged into a chiral superstructure. Notably, the chiral superstructure shows strong optical activity due to the difference of absorbing left- and right-handed circularly polarized light. This special optical activity resulted from electron transition from the valence band to the conduction band of TiO(2) through a vicinal effect of helically arranged TiO(2) nanocrystals.

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