Fate of charge order in overdoped La-based cuprates

过掺杂镧基铜酸盐中电荷有序的演变

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Abstract

In high-temperature cuprate superconductors, stripe order refers broadly to a coupled spin and charge modulation with a commensuration of eight and four lattice units, respectively. How this stripe order evolves across optimal doping remains a controversial question. Here we present a systematic resonant inelastic x-ray scattering study of weak charge correlations in La(2-x)Sr(x)CuO(4) and La(1.8-x)Eu(0.2)Sr(x)CuO(4). Ultra high energy resolution experiments demonstrate the importance of the separation of inelastic and elastic scattering processes. Long-range temperature-dependent stripe order is only found below optimal doping. At higher doping, short-range temperature-independent correlations are present up to the highest doping measured. This transformation is distinct from and preempts the pseudogap critical doping. We argue that the doping and temperature-independent short-range correlations originate from unresolved electron-phonon coupling that broadly peaks at the stripe ordering vector. In La(2-x)Sr(x)CuO(4), long-range static stripe order vanishes around optimal doping and we discuss both quantum critical and crossover scenarios.

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