First-Principles Study of the Ga(2)O(3)/Metal Interface by Inserting a Boron Nitride Monolayer

通过插入氮化硼单层对 Ga(2)O(3)/金属界面进行第一性原理研究

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Abstract

The wide band gap semiconductor Ga(2)O(3) has been well studied in terms of the Schottky diodes. Controlling the Schottky barrier height (SBH) in Ga(2)O(3)/metal contacts is essential for achieving desirable, high-performance electronic devices. In this article, based on first-principles calculations, we studied the effect of inserting a two-dimensional dielectric layer of hexagonal boron nitride (h-BN) on the SBH of Ga(2)O(3)/metal. Two sets of interface models with and without the BN interlayer, i.e., Ga(2)O(3)/Au, Ga(2)O(3)/BN/Au, Ga(2)O(3)/Mg, and Ga(2)O(3)/BN/Mg configurations, were built. As a result, the SBH of high metal work function Au interfaces does not show a significant change after h-BN insertion. In contrast, the SBH of low metal work function Mg interfaces was increased significantly by an h-BN insertion. The reason for this at the atomic level was also explained through electronic structure calculations. They show that inducing a two-dimensional h-BN monolayer can be seen as a transition layer to screen the interface states effectively and weaken the interface interaction greatly. Besides, the effect of the h-BN interlayer on the tunneling barriers was also analyzed. We believe this study will provide insight into improving the performance of wide band gap semiconductor devices with an intercalation structure.

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