Synthesis and photocatalytic activity of mesoporous g-C(3)N(4)/MoS(2) hybrid catalysts

介孔gC(3)N(4)/MoS(2)杂化催化剂的合成及光催化活性

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Abstract

The key to solving environmental and energy issues through photocatalytic technology requires highly efficient, stable and eco-friendly photocatalysts. Graphitic carbon nitride (g-C(3)N(4)) is one of the most promising candidates except for its limited photoactivity. In this work, a facile and scalable one-step method is developed to fabricate an efficient heterostructural g-C(3)N(4) photocatalyst in situ coupled with MoS(2). The strong coupling effect between the MoS(2) nanosheets and g-C(3)N(4) scaffold, numerous mesopores and enlarged specific surface area helped form an effective heterojunction. As such, the photocatalytic activity of the g-C(3)N(4)/MoS(2) is more than three times higher than that of the pure g-C(3)N(4) in the degradation of RhB under visible light irradiation. Improvement of g-C(3)N(4)/MoS(2) photocatalytic performance is mainly ascribed to the effective suppression of the recombination of charge carriers.

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