Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions

聚合物溶液中混合的时间相关自聚焦和散焦非线性

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作者:Athanasios Bogris, Nikolaos A Burger, Konstantinos G Makris, Benoit Loppinet, George Fytas

Abstract

Low-power visible light can lead to spectacular nonlinear effects in soft-matter systems. The propagation of visible light through transparent solutions of certain polymers can experience either self-focusing or defocusing nonlinearity, depending on the solvent. We show how the self-focusing and defocusing responses can be captured by a nonlinear propagation model using local spatial and time-integrating responses. We realize a remarkable pattern formation in ternary solutions and model it assuming a linear combination of the self-focusing and defocusing nonlinearities in the constituent solvents. This versatile response of solutions to light irradiation may introduce a new approach for self-written waveguides and patterns.

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