Influence of Available Hydrophobic Interactions in New 2‑(Propylthio)‑N‑(1,3,4-thiadiazol-2-yl)nicotinamide Pharmacophore and Evaluation of Its Therapeutic Potential

新型2-(丙基硫代)-N-(1,3,4-噻二唑-2-基)烟酰胺药效团中可用疏水相互作用的影响及其治疗潜力的评价

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Abstract

Required hydrophobic interactions exerted by the new pharmacophore 2-(propylthio)-N-(1,3,4-thiadiazol-2-yl)-nicotinamide (Compound 3) were designed, synthesized, and characterized by NMR, FFT-IR, high-resolution mass spectrometry (HR-MS), and single-crystal X-ray diffraction (SC-XRD) analytical techniques. Based on the SC-XRD analysis, the pharmacophore's surface characteristics were evaluated by Hirshfield surface analysis, and it was compared with the theoretical DFT-optimized structure. This demonstrates the structural overview of nucleophilic and electrophilic parts and the molecular electrostatic potential values in the range of -0.05547 to +0.05547. The Compound 3 drug-likeness property was validated by in silico techniques. From the molecular docking study, compound 3 has binding interactions of -7.82 kcal/mol with COX-1 and -7.08 kcal/mol with COX-2 isoforms of the cyclooxygenase enzyme. Compound 3 was explored for free-radical scavenging activity by ABTS and DPPH assays. Further, its bioefficacy was validated by using the MTT cell viability assay, COX-2, and LOX-5 enzyme inhibition. Then, the Compound 3 antibacterial efficiency was also examined by the Gram-negative and Gram-positive bacterial strains. Combining the above results, this study offers insights into the hydrophobic nature of new pharmacophore motifs and their impactful effects on biological properties.

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