Discovery of Prodrug of MRTX1133 as an Oral Therapy for Cancers with KRAS(G12D) Mutation

发现MRTX1133前药作为KRAS(G12D)突变癌症的口服疗法

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Abstract

Effective oral therapies are urgently required to treat KRAS(G12D) mutant cancers. Therefore, synthesis and screening were performed for 38 prodrugs of MRTX1133 to identify an oral prodrug of MRTX1133, a KRAS(G12D) mutant protein-specific inhibitor. In vitro and in vivo evaluations revealed prodrug 9 as the first orally available KRAS(G12D) inhibitor. Prodrug 9 exhibited improved pharmacokinetic properties for the parent compound in mice and was efficacious in a KRAS(G12D) mutant xenograft mouse tumor model after oral administration.

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